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ISA-YMG粗铅冶炼新工艺

王吉坤,周廷熙,冯桂林

《中国工程科学》 2004年 第6卷 第4期   页码 61-66

摘要：

评述了铅提取技术的历史及现代铅提取技术的特点；针对我国目前粗铅冶炼现状，结合对高铅渣冶炼的多年研究，提出一种高效、节能、清洁的ISA-YMG粗铅冶炼新工艺，并提供了YMG还原熔炼工业试验结果。

关键词： 铅ISA氧化熔炼     高铅渣     铅YMG还原熔炼     粗铅冶炼新工艺    

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Modeling limit force capacities of high force to volume lead extrusion dampers

《结构与土木工程前沿（英文）》 2021年 第15卷 第3期   页码 609-622 doi: 10.1007/s11709-021-0724-x

摘要： Lead extrusion dampers are supplemental energy-dissipation devices that are used to mitigate seismic structural damage. Small volumetric sizes and high force capacities define high-force-to-volume (HF2V) devices, which can absorb significant response energy without sacrificial damage. However, the design of such devices for specific force capacities has proven difficult based on the complexities of their internal reaction mechanisms, leading to the adoption of empirical approaches. This study developed upper- and lower-bound force capacity estimates from analytical mechanics based on direct and indirect metal extrusion for guiding design. The derived equations are strictly functions of HF2V device geometric parameters, lead material properties, and extrusion mechanics. The upper-bound estimates from direct and indirect extrusion are denoted as (FUB,1, FUB,2) and (FUB,3, FUB,4), respectively, and the lower-bound estimates are denoted as (FLB, FLB,1) based on the combination of extrusion and friction forces. The proposed models were validated by comparing the predicted bounds to experimental force capacity data from 15 experimental HF2V device tests. The experimental device forces all lie above the lower-bound estimates (FLB, FLB,1) and below the upper-bound estimates (FUB,1, FUB,2, FUB,4). Overall, the (FLB, FUB,2) pair provides wider bounds and the (FLB,1, FUB,4/FUB,1) pair provides narrower bounds. The (FLB,1, FUB,1) pair has a mean lower-bound gap of 36%, meaning the lower bound was 74% of the actual device force on average. The mean upper-bound gap was 33%. The bulge area and cylinder diameter of HF2V devices are key parameters affecting device forces. These relatively tight bounds provide useful mechanics-based predictive design guides for ensuring that device forces are within the targeted design range after manufacturing.

关键词： extrusion     lead dampers     upper and lower bound     analytical modelling     limit force    

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Removal of lead from aqueous solution by hydroxyapatite/manganese dioxide composite

Lijing DONG,Zhiliang ZHU,Yanling QIU,Jianfu ZHAO

《环境科学与工程前沿（英文）》 2016年 第10卷 第1期   页码 28-36 doi: 10.1007/s11783-014-0722-5

摘要： A novel composite adsorbent, hydroxyapatite/manganese dioxide (HAp/MnO ), has been developed for the purpose of removing lead ions from aqueous solutions. The combination of HAp with MnO is meant to increase its adsorption capacity. Various factors that may affect the adsorption efficiency, including solution pH, coexistent substances such as humic acid and competing cations (Ca , Mg ), initial solute concentration, and the duration of the reaction, have been investigated. Using this composite adsorbent, solution pH and coexistent calcium or magnesium cations were found to have no significant influence on the removal of lead ions under the experimental conditions. The adsorption equilibrium was described well by the Langmuir isotherm model, and the calculated maximum adsorption capacity was 769 mg·g . The sorption processes obeyed the pseudo-second-order kinetics model. The experimental results indicate that HAp/MnO composite may be an effective adsorbent for the removal of lead ions from aqueous solutions.

关键词： lead     composite materials     manganese dioxide     hydroxyapatite     adsorption    

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Biosorption of mercury and lead by aqueous

Pratibha SANJENBAM, Kumar SAURAV, Krishnan KANNABIRAN

《化学科学与工程前沿（英文）》 2012年 第6卷 第2期   页码 198-202 doi: 10.1007/s11705-012-1285-2

摘要： Toxic heavy metals are increasingly accumulating in the environment worldwide and are considered to be life threatening contaminants. The biosorption of mercury and lead by marine actinomycetes isolated from marine sediment collected from the Bay of Bengal coast of Puducherry, India, was evaluated. The maximum tolerance concentration (MTC) of sp. was determined by a well diffusion method and a broth dilution method. The effects of the initial metal ion concentration, the pH and the biomass dosage on the biosorption of mercury and lead ions were investigated. The MTC of the isolate to metals was 200 mg·L for mercury and 1800 mg·L for lead. At neutral pH, the isolate had a maximum biosorption of metal ions of 200 mg·L and 150 mg·L for mercury and lead respectively. Fourier transform infrared (FTIR) absorption spectra showed the chemical interactions between the functional groups in the biomass such as hydroxyl (-OH), amine (-NH ), carboxyl (-COOH) and the metal ions. The isolate was further characterized by molecular taxonomy and identified as a member of the genus Based on the phenotypic and phylogenetic analysis, the strain was classified as a new species of the genus and designated as VITSVK9 sp. (HM137310). A blast search of the 16S rDNA sequence of the strain showed the most similarity (95%) with sp. A515 Ydz-FQ (EU384279). Based on the results, it can be concluded that this marine could be used as a biosorbent for the removal of heavy metal ions from aqueous environments.

关键词： mercury     lead     biosorption     maximum tolerance concentration     Streptomyces VITSVK9 sp.    

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Performance and mechanism for cadmium and lead adsorption from water and soil by corn straw biochar

Tong Chi,Jiane Zuo,Fenglin Liu

《环境科学与工程前沿（英文）》 2017年 第11卷 第2期 doi: 10.1007/s11783-017-0921-y

摘要： Corn straw biochar prepared under 400 °C was the best Cd and Pb adsorption capacity Maximum adsorption capacity of Cd and Pb were 43.48 and 22.73 mg·g , respectively The dominant mechanism of Cd and Pb adsorption was precipitation Biochar could reduce the bioavailability of heavy metals when mixed with soil Cadmium (Cd) and lead (Pb) in water and soil could be adsorbed by biochar produced from corn straw. Biochar pyrolyzed under 400°C for 2 h could reach the ideal removal efficiencies (99.24% and 98.62% for Cd and Pb, respectively) from water with the biochar dosage of 20 g·L and initial concentration of 20 mg·L . The pH value of 4–7 was the optimal range for adsorption reaction. The adsorption mechanism was discussed on the basis of a range of characterizations, including X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), Fourier transform infrared spectroscopy (FTIR) and Raman analysis; it was concluded as surface complexation with active sorption sites (-OH, -COO-), coordination with π electrons (C= C, C= O) and precipitation with inorganic anions (OH , CO , SO ) for both Cd and Pb. The sorption isotherms fit Langmuir model rather than Freundlich model, and the saturated sorption capacities for Cd and Pb were 38.91 mg·g and 28.99 mg·g , respectively. When mixed with soil, biochar could effectively increase alkalinity and reduce bioavailability of heavy metals. Thus, biochar derived from corn straw would be a green material for both removal of heavy metals and amelioration of soil.

关键词： Corn straw     Biochar     Heavy metals     Sorption isotherm     Bioavailability    

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Effects of nano-silicon and common silicon on lead uptake and translocation in two rice cultivars

Jianguo LIU,Hui CAI,Congcong MEI,Mingxin WANG

《环境科学与工程前沿（英文）》 2015年 第9卷 第5期   页码 905-911 doi: 10.1007/s11783-015-0786-x

摘要： The current study investigated the effects of nano-silicon (Si) and common Si on lead (Pb) toxicity, uptake, translocation, and accumulation in the rice cultivars Yangdao 6 and Yu 44 grown in soil containing two different Pb levels (500 mg·kg and 1000 mg·kg ). The results showed that Si application alleviated the toxic effects of Pb on rice growth. Under soil Pb treatments of 500 and 1000 mg·kg , the biomasses of plants supplied with common Si and nano-Si were 1.8%–5.2% and 3.3%–11.8% higher, respectively, than those of plants with no Si supply (control). Compared to the control, Pb concentrations in rice shoots supplied with common Si and nano-Si were reduced by 14.3%–31.4% and 27.6%–54.0%, respectively. Pb concentrations in rice grains treated with common Si and nano-Si decreased by 21.3%–40.9% and 38.6%–64.8%, respectively. Pb translocation factors (TFs) from roots to shoots decreased by 15.0%–29.3% and 25.6%–50.8%, respectively. The TFs from shoots to grains reduced by 8.3%–13.7% and 15.3%–21.1%, respectively, after Si application. The magnitudes of the effects observed on plants decreased in the following order: nano-Si treatment>common Si treatment and high-grain-Pb-accumulating cultivar (Yangdao 6)>low-grain-Pb-accumulating cultivar (Yu 44) and heavy Pb stress (1000 mg·kg )>moderate Pb stress (500 mg·kg )>no Pb treatment. The results of the study indicate that nano-Si is more efficient than common Si in ameliorating the toxic effects of Pb on rice growth, preventing Pb transfer from rice roots to aboveground parts, and blocking Pb accumulation in rice grains, especially in high-Pb-accumulating rice cultivars and in heavily Pb-polluted soils.

关键词： silicon (Si)     lead (Pb)     rice (Oryza sativa L.)     toxicity     accumulation    

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中国ADS 铅基反应堆设计与研发进展 Review

吴宜灿

《工程（英文）》 2016年 第2卷 第1期   页码 124-131 doi: 10.1016/J.ENG.2016.01.023

摘要：

2011年，在中国科学院战略性先导专项“未来先进核裂变能——加速器驱动次临界嬗变系统”等项目的支持下，针对加速器驱动次临界系统和第四代铅冷快堆的技术发展目标和试验要求，完成了具有临界和加速器驱动次临界双模式运行能力的10 MW中国铅基研究堆CLEAR-I的概念设计，建成了KYLIN系列铅铋回路试验平台，并在此基础上开展了反应堆冷却剂技术、关键组件、结构材料与燃料、反应堆运行与控制技术等铅铋反应堆关键技术的研发。为验证及测试铅基堆关键组件和综合操作技术，正在开展铅合金冷却非核反应堆CLEAR-S、铅基零功率核反应堆CLEAR-0和铅基虚拟反应堆CLEAR-V的建设。

关键词： 加速器驱动次临界系统     中国铅基反应堆     铅铋共晶     技术研发进展    

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Competitive adsorption and desorption of copper and lead in some soil of North China

Fengjie ZHANG, Xiaoxia OU, Shuo CHEN, Chunqiu RAN, Xie QUAN

《环境科学与工程前沿（英文）》 2012年 第6卷 第4期   页码 484-492 doi: 10.1007/s11783-012-0423-x

摘要： The competitive adsorption and desorption of Pb(II) and Cu(II) ions in the soil of three sites in North China were investigated using single and binary metal solutions with 0.01 mol·L CaCl as background electrolyte. The desorption isotherms of Pb(II) and Cu(II) were similar to the adsorption isotherms, which can be fitted well by Freundlich equation ( >0.96). The soil in the three sites had greater sorption capacities for Pb(II) than Cu(II), which was affected strongly by the soil characteristics. In the binary metal solution containing 1∶1 molar ratio of Pb(II) and Cu(II), the total amount of Pb(II) and Cu(II) adsorption was affected by the simultaneous presence of the two metal ions, indicating the existence of adsorption competition between the two metal ions. Fourier transform infrared (FT-IR) spectroscopy was used to investigate the interaction between soil and metal ions, and the results revealed that the carboxyl and hydroxyl groups in the soil were the main binding sites of metal ions.

关键词： competitive adsorption     desorption     copper     lead     soil    

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Model test study for ice force on the bank-head of the lead-navigating bank

SONG An, SUN Jinliang, LU Hai, WANG Yi′an

《结构与土木工程前沿（英文）》 2007年 第1卷 第2期   页码 222-228 doi: 10.1007/s11709-007-0027-x

摘要： To determine the bank-head s ice force of the lead-navigating bank at key position that faces the ice directly of certain water conservancy, ice model test in reduced scale is designed and carried out based on the local situation on the spot and data observed. Preliminary conclusions are got through the analysis of the experimental data such as effect of the ice velocity on the ice force , ratio of components of forces when ice sheet acting on the vertical bank-head, ice force ratio of vertical to 45? incline as well as ratio of level ice force to the vertical ice force when acting on 45? incline. Finally, suggestions on determination of the ice force using formula are given after comparison between the result calculated by the present formula of ice force and the experimental results.

关键词： comparison     lead-navigating bank     vertical bank-head     certain     Preliminary    

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fabricating photoluminescent carbon dots and its potential application as an efficient sensor probe for toxic lead

《化学科学与工程前沿（英文）》 2023年 第17卷 第5期   页码 536-547 doi: 10.1007/s11705-022-2239-y

摘要： The past decade has witnessed a variety of members of the carbon family along with exposure of carbon dots due to their magnificent properties in sensing, bioimaging, catalytic applications, biomedical fields, and so on. Herein, we report the simple hydrothermal method to fabricate photoluminescent doped carbon quantum dots for the detection of noxious lead(II) ions. Lead(II) ion is very venomous for both the environment and human health for which its detection is demanded area in the research field. The as-prepared carbon dots show excellent photostability, low toxicity and significant photoluminescence properties along with good water solubility. Along with these properties, carbon dots have a quantum yield of approximately 15%. In the practical field of application, these carbon dots have been used as sensing probes for the detection of lead(II) ions with a detection limit of 60 nmol·L–1. The fluorescence intensity of carbon dots was remarkably quenched in the presence of the lead(II) ion selectively among all the tested metal ions. Furthermore, we have studied the Stern–Volmer relationship for lead(II) quenching along with the explanation of the probable quenching mechanism. Ability of the doped carbon dots in heavy metal ions sensing in an environmental sample was demonstrated.

关键词： carbon dots     fluorescence     heavy metal sensing     practical application     photoluminescence    

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Genotype variations in accumulation of cadmium and lead in celery (

Kun ZHANG, Jianbing WANG, Zhongyi YANG, Guorong XIN, Jiangang YUAN, Junliang XIN, Charlie HUANG

《环境科学与工程前沿（英文）》 2013年 第7卷 第1期   页码 85-96 doi: 10.1007/s11783-012-0399-3

摘要： To help reduce risks of heavy metal pollution, two pot experiments were conducted to investigate the variations, transfer potential, and stability of Cadmium (Cd) and Lead (Pb) accumulations in celery ( L.) and to screen for low Cd and Pb accumulative cultivars. The maximum differences in shoot Cd concentration were 4.7-fold under low-Cd exposure and 3.3-fold under high-Cd exposure. These genotype variations in Cd accumulation are sufficiently large to help reduce Cd contamination risk in soil by using the Low-Cd-Accumulative genotypes. Cd accumulation of the Low-Cd-Accumulative genotypes is significantly positive correlated with Pb accumulation. Evidence obtained proves that Cd and Pb accumulations in celery are stable and genotype-dependent at the cultivar level. The presence of high-Pb contamination in soil promoted Cd accumulation in shoots of celery. Celery is considered a species with high risks in Cd pollution and low risks in Pb pollution. Among the tested cultivars, cv. Shuanggangkangbing (SGKB) had the lowest shoot Cd and Pb accumulating abilities, and thus is the most important material for breeding of pollution-safe cultivars (PSCs) to minimize Cd and Pb accumulations in celery.

关键词： cadmium (Cd) accumulation     lead (Pb) accumulation     celery     genotype variation     food safety    

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Low-carbohydrate diets lead to greater weight loss and better glucose homeostasis than exercise: a randomized

《医学前沿（英文）》 2021年 第15卷 第3期   页码 460-471 doi: 10.1007/s11684-021-0861-6

摘要： Lifestyle interventions, including dietary adjustments and exercise, are important for obesity management. This study enrolled adults with overweight or obesity to explore whether either low-carbohydrate diet (LCD) or exercise is more effective in metabolism improvement. Forty-five eligible subjects were randomly divided into an LCD group (n=22) and an exercise group (EX, n=23). The subjects either adopted LCD (carbohydrate intake<50 g/day) or performed moderate-to-vigorous exercise (≥30 min/day) for 3 weeks. After the interventions, LCD led to a larger weight loss than EX (−3.56±0.37 kg vs. −1.24±0.39 kg, P<0.001), as well as a larger reduction in fat mass (−2.10±0.18 kg vs. −1.25±0.24 kg, P=0.007) and waist circumference (−5.25±0.52 cm vs. −3.45±0.38 cm, P=0.008). Both interventions reduced visceral and subcutaneous fat and improved liver steatosis and insulin resistance. Triglycerides decreased in both two groups, whereas low-density lipoprotein cholesterol increased in the LCD group but decreased in the EX group. Various glycemic parameters, including serum glycated albumin, mean sensor glucose, coefficient of variability (CV), and largest amplitude of glycemic excursions, substantially declined in the LCD group. Only CV slightly decreased after exercise. This pilot study suggested that the effects of LCD and exercise are similar in alleviating liver steatosis and insulin resistance. Compared with exercise, LCD might be more efficient for weight loss and glucose homeostasis in people with obesity.

关键词： low-carbohydrate diet     obesity     nonalcoholic fatty liver disease     continuous glucose monitoring     mean sensor glucose    

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Long-lasting photoluminescence quantum yield of cesium lead halide perovskite-type quantum dots

Yonghyun Kim, Huiwen Liu, Yi Liu, Boa Jin, Hao Zhang, Wenjing Tian, Chan Im

《化学科学与工程前沿（英文）》 2021年 第15卷 第1期   页码 187-197 doi: 10.1007/s11705-020-1931-z

摘要： Cesium lead halide perovskite (CsPbX , X= Cl, Br, I) quantum dots (QDs) and their partly Mn -substituted QDs (CsPb Mn X ) attract considerable attention owing to their unique photoluminescence (PL) efficiencies. The two types of QDs, having different PL decay dynamics, needed to be further investigated in a form of aggregates to understand their solid-state-induced exciton dynamics in conjunction with their behaviors upon degradation to achieve practical applications of those promising QDs. However, thus far, these QDs have not been sufficiently investigated to obtain deep insights related to the long-term stability of their PL properties as aggregated solid-states. Therefore, in this study, we comparatively examined CsPbX - and CsPb Mn X -type QDs stocked for>50 d under dark ambient conditions by using excitation wavelength-dependent PL quantum yield and time-resolved PL spectroscopy. These investigations were performed with powder samples in addition to solutions to determine the influence of the inter-QD interaction of the aged QD aggregates on their radiative decays. It turns out that the Mn -substituted QDs exhibited long-lasting PL quantum efficiencies, while the unsubstituted CsPbX -type QDs exhibited a drastic reduction of their PL efficiencies. And the obtained PL traces were clearly sensitive to the sample status. This is discussed with the possible interaction depending on the size and distance of the QD aggregates.

关键词： quantum dots     cesium lead halide perovskite     time-resolved photoluminescence     PL quantum yield     QD aggregates    

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Cadmium and lead toxicity and bioaccumulation in

RZYMSKI Piotr,PONIEDZIALEK Barbara,NIEDZIELSKI Przemysław,TABACZEWSKI Piotr,WIKTOROWICZ Krzysztof

《环境科学与工程前沿（英文）》 2014年 第8卷 第3期   页码 427-432 doi: 10.1007/s11783-013-0566-4

摘要： The growth of human population leads to intensification of agriculture and promotes, through eutrophication, development of cyanobacteria. One of the most widespread and bloom-forming species in freshwater is toxic ( ). Combustion of fossil fuels and metallurgical processes are the main sources of heavy metals contamination in surface water including cadmium (Cd) and lead (Pb). The following study was conducted in order to determine the effect of 1–20 mg·L of Cd and Pb on photochemistry (using flow cytometry) and growth (based on chlorophyll concentration) of as well as to estimate levels of metal bioaccumulation. We have found that 1–10 mg·L of Cd and 1–5 mg·L of Pb induced continuous enhancement of chlorophyll fluorescence during 24 h of incubation. No significant degradation of chlorophyll was observed in these samples. At higher concentrations of 20 mg·L of Cd and 10–20 mg·L of Pb chlorophyll level significantly decreased and its fluorescence was quenched. demonstrated high capability of Cd and Pb bioaccumulation, proportionally to initial metal concentration. In samples with initial concentration of 20 mg·L of Cd and Pb bioaccumulation of 87.3% and 90.1% was observed, respectively. Our study demonstrates that can potentially survive in highly metals polluted environments, be a primary source of toxic metals in the food chain and consequently contribute to enhanced toxicity of heavy metals to living organisms including human.

关键词： Microcystis aeruginosa     heavy metals     bioaccumulation     chlorophyll     flow cytometry    

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Algae (

Xuesong Liu, Jianmin Wang

《环境科学与工程前沿（英文）》 2020年 第14卷 第6期 doi: 10.1007/s11783-020-1276-3

摘要： Abstract • Micro-plastics (MPs) significantly increase Pb toxicity. • Algae reduce the combined toxicity of MP and Pb. • The toxicity increase comes from high soluble Pb and MP-Pb uptake. • The toxicity reduction might come from energy related pathway. Microplastics (MPs) have been recognized as a new class of emerging contaminants in recent years. They not only directly impact aquatic organisms, but also indirectly impact these organisms by interacting with background toxins in the environment. Moreover, under realistic environmental conditions, algae, a natural food for aquatic organisms, may alter the toxicity pattern related to MPs. In this research, we first examined the toxicity of MPs alone, and their effect on the toxicity of lead (Pb) on Ceriodaphnia dubia (C. dubia), a model aquatic organism for toxicity survey. Then, we investigated the effect of algae on the combined toxicity of MPs and Pb. We observed that, MPs significantly increased Pb toxicity, which was related to the increase in soluble Pb concentration and the intake of Pb-loaded MPs, both of which increased the accumulation of Pb in C. dubia. The presence of algae mitigated the combined toxicity of MPs and Pb, although algae alone increased Pb accumulation. Therefore, the toxicity mitigation through algae uptake came from mechanisms other than Pb accumulation, which will need further investigation.

关键词： Microplastic     Lead     Toxicity     Algae     C. dubia    

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标题 作者 时间 类型 操作

ISA-YMG粗铅冶炼新工艺

王吉坤,周廷熙,冯桂林

期刊论文

Modeling limit force capacities of high force to volume lead extrusion dampers

期刊论文

Removal of lead from aqueous solution by hydroxyapatite/manganese dioxide composite

Lijing DONG,Zhiliang ZHU,Yanling QIU,Jianfu ZHAO

期刊论文

Biosorption of mercury and lead by aqueous

Pratibha SANJENBAM, Kumar SAURAV, Krishnan KANNABIRAN

期刊论文

Performance and mechanism for cadmium and lead adsorption from water and soil by corn straw biochar

Tong Chi,Jiane Zuo,Fenglin Liu

期刊论文

Effects of nano-silicon and common silicon on lead uptake and translocation in two rice cultivars

Jianguo LIU,Hui CAI,Congcong MEI,Mingxin WANG

期刊论文

中国ADS 铅基反应堆设计与研发进展

吴宜灿

期刊论文

Competitive adsorption and desorption of copper and lead in some soil of North China

Fengjie ZHANG, Xiaoxia OU, Shuo CHEN, Chunqiu RAN, Xie QUAN

期刊论文

Model test study for ice force on the bank-head of the lead-navigating bank

SONG An, SUN Jinliang, LU Hai, WANG Yi′an

期刊论文

fabricating photoluminescent carbon dots and its potential application as an efficient sensor probe for toxic lead

期刊论文

Genotype variations in accumulation of cadmium and lead in celery (

Kun ZHANG, Jianbing WANG, Zhongyi YANG, Guorong XIN, Jiangang YUAN, Junliang XIN, Charlie HUANG

期刊论文

Low-carbohydrate diets lead to greater weight loss and better glucose homeostasis than exercise: a randomized

期刊论文

Long-lasting photoluminescence quantum yield of cesium lead halide perovskite-type quantum dots

Yonghyun Kim, Huiwen Liu, Yi Liu, Boa Jin, Hao Zhang, Wenjing Tian, Chan Im

期刊论文

Cadmium and lead toxicity and bioaccumulation in

RZYMSKI Piotr,PONIEDZIALEK Barbara,NIEDZIELSKI Przemysław,TABACZEWSKI Piotr,WIKTOROWICZ Krzysztof

期刊论文

Algae (

Xuesong Liu, Jianmin Wang

期刊论文